[PDF] Toward High Performance Broad Band Frequency Comb Operation Of Terahertz Quantum Cascade Lasers eBook

Author : Chao Xu
Publisher :
Page : 128 pages
File Size : 35,2 MB
Release : 2017
Category : Lasers
ISBN :

GET BOOK

Recent advances in Terahertz Quantum Cascade Laser (THz QCL) development are pushing this technology ever closer to practical application, particularly within the spectroscopic field. For this reason, optimizing the operation of THz QCL frequency combs, which can potentially provide unprecedented accuracy and stability to the optical spectra in a broad frequency band, is of particular interest to the research community. The THz QCLs frequency comb was only recently realized using two separate techniques: either a broad-gain active region or a group velocity dispersion controlled waveguide. However, due to residual optical dispersion from both the gain medium and the cold waveguide, comb formation in these reported THz QCLs can only sustain a limited current injection region and the observed comb frequency range is much narrower than the bandwidth of the designed gain medium. To overcome these limitations, this thesis targets a new THz QCL frequency comb device design that simultaneously exploits the broadband gain active region and a group velocity dispersion (GVD)-compensated waveguide over an octave frequency band of 2-4 THz. In designing a broadband gain active region, two heterogeneous structures are proposed and simulated, with one combining three different bound-to-continuum (BTC) active regions operating at a temperature of 25 K, and another one consisting of four different resonant-phonon (RP) active regions operating at the liquid nitrogen temperature (77 K) or higher. The simulation results show that both active region designs can provide a broadband and 'flat-top' gain profile covering the frequency range from 2 to 4 THz. To design a group velocity dispersion-compensated waveguide, strategies are explored for simulating chirped Distributed Bragg Reflectors (DBRs) that can serve as THz QCL metal-metal waveguides, and one-dimensional (1D) and three-dimensional (3D) modeling approaches are established and verified. A novel two-section chirped DBR is proposed, which provides substantially-improved group delay compensation over a broadband octave frequency range from 2 to 4 THz. Two THz QCL structures are grown using in-house molecular beam epitaxy and THz QCL devices equipped with a metal-metal waveguides are fabricated in the University of Waterloo Quantum-Nano-Centre clean-room fabrication lab. The experimental results demonstrate that the new THz QCL active region design can operate up to a maximum lasing temperature of 111 K, and with a broad lasing spectrum covering frequencies from 2.36 to 2.86 THz under pulse mode, at temperature of 13 K. The combined theoretical and experimental work would ultimately lead to the demonstration of improved THz QCL frequency comb operation over the broadband range from 2 to 4 THz.

Author : Yang Yang (Ph. D.)
Publisher :
Page : 162 pages
File Size : 39,5 MB
Release : 2019
Category :
ISBN :

GET BOOK

In recent years, there has been growing interest in chip-scale frequency combs, such as micro-resonator combs and semiconductor mode-locked sources. From the mid-infrared to the terahertz regime, it has been shown that quantum cascade lasers (QCLs) are capable of forming a frequency comb state where dispersed cavity modes of the Fabry-Perot cavity are synchronized by third order nonlinearity. With proper dispersion engineering, we have shown that it is possible to create QCL frequency combs at terahertz wavelengths, which possess broadband coverage in a compact package. These QCL combs are particularly attractive as sources for high-sensitivity laser spectroscopy: by using a dual-comb technique, it is possible to perform broadband spectroscopy only using chip-scale components, making it an intriguing candidate for spectroscopic applications in the open field. Moreover, due to the semi-continuous nature of the temporal output from such combs, tracking the instantaneous phase and timing signals of the dual-comb waveform in the time domain becomes feasible. This enables a computational coherent averaging scheme of the dual-comb signal even without external reference. The first part of this thesis describes the development for better THz laser frequency combs. To realize all expectations in the spectroscopy applications using such devices, three main aspects of improvement are highly desired. First, the laser device should have a robust comb state that ideally can operate from device's threshold current, I[subscript th], to its maximum current, I[subscript m]. In addition, the comb states should have a broad spectral coverage: its bandwidth should cover at least an octave span to stabilize its carrier offset. Furthermore, the comb state should have a flexible tunability that allows tuning across the entire free spectral range for gapless sensing. All listed aspects are investigated during the course of this thesis and as a result, a THz QCL device featuring comb state performance over the entire lasing bias range has been demonstrated. Meanwhile, we show that, by compensating cavity dispersion up to higher orders, the comb bandwidth from the full dispersion compensated devices can reach 80 % of its gain bandwidth. One common method to achieve very broadband coverage relies on using the heterogeneous gain media. This comes at the cost of reduced peak gain and hampered temperature performance. Also, engineering the dispersion of such a broadband gain medium becomes extremely challenging, which might not lead to a broader comb coverage albeit its broader gain. However, a unique feature of the metal-metal waveguide is that it is completely agnostic about its bonded gain media. Therefore, it is possible to bond multiple gain media together onto the same chip. The lateral heterogeneous integration scheme is investigated as an alternative method to expand the comb's spectral coverage. We show that using this strategy we can couple the output of combs at vastly different wavelengths without the trade-off with its temperature performance, yet maintain a compact package. Dual-comb spectroscopy allows for high-resolution spectra to be measured over broad bandwidth, but in order to achieve high resolution and acquire low-uncertainty spectroscopic information, the capability for coherent averaging is of the most importance. An essential requirement for coherent averaging is the availability of a phase reference. Usually, this means that the combs' phase and timing errors must be measured and either minimized by stabilization or removed by correction. These hardware-based solutions often require extra electronic or optical components, thus complicates the overall system and further limits the technique's applicability. We demonstrate that it is possible to extract the phase and timing signals of a multiheterodyne spectrum in a completely computational fashion without any extra measurements, which can potentially simplify any dual-comb system. Other works in this thesis include the first proof-of-principle demonstration of THz dual-comb spectroscopy using laser frequency combs, THz hyper-spectral imaging for pharmaceutical compound identification, and the exploratory work on the development of the germanium-on-gallium arsenide platform, a passive on-chip platform showing potential to bridge the THz and mid-infrared regime.

Author : Tasmim Alam
Publisher : Cuvillier Verlag
Page : 132 pages
File Size : 17,41 MB
Release : 2020-10-29
Category : Science
ISBN : 3736962975

GET BOOK

Quantum cascade lasers (QCLs) are attractive for high-resolution spectroscopy because they can provide high power and a narrow linewidth. They are particularly promising in the terahertz (THz) range since they can be used as local oscillators for heterodyne detection as well as transmitters for direct detection. However, THz QCL-based technologies are still under development and are limited by the lack of frequency tunability as well as the frequency and output power stability for free-running operation. In this dissertation, frequency tuning and linewidth of THz QCLs are studied in detail by using rotational spectroscopic features of molecular species. In molecular spectroscopy, the Doppler eff ect broadens the spectral lines of molecules in the gas phase at thermal equilibrium. Saturated absorption spectroscopy has been performed that allows for sub-Doppler resolution of the spectral features. One possible application is QCL frequency stabilization based on the Lamb dip. Since the tunability of the emission frequency is an essential requirement to use THz QCL for high-resolution spectroscopy, a new method has been developed that relies on near-infrared (NIR) optical excitation of the QCL rear-facet. A wide tuning range has been achieved by using this approach. The scheme is straightforward to implement, and the approach can be readily applied to a large class of THz QCLs. The frequency and output stability of the local oscillator has a direct impact on the performance and consistency of the heterodyne spectroscopy. A technique has been developed for a simultaneous stabilization of the frequency and output power by taking advantage of the frequency and power regulation by NIR excitation. The results presented in this thesis will enable the routine use of THz QCLs for spectroscopic applications in the near future.

Author : Dan Botez
Publisher : Cambridge University Press
Page : 552 pages
File Size : 49,49 MB
Release : 2023-09-14
Category : Technology & Engineering
ISBN : 1108570607

GET BOOK

Learn how the rapidly expanding area of mid-infrared and terahertz photonics has been revolutionized in this comprehensive overview. State-of-the-art practical applications are supported by real-life examples and expert guidance. Also featuring fundamental theory enabling you to improve performance of both existing and future devices.

Author : Yu Wu
Publisher :
Page : 0 pages
File Size : 11,73 MB
Release : 2023
Category :
ISBN :

GET BOOK

The invention of optical frequency combs generated by mode-locked lasers revolutionized time and frequency metrology in the late 1990s. This concept has been explored in several laser systems; the quantum cascade laser (QCL) is one such system that operates in the terahertz (THz) frequency range.THz QCL was first invented in 2001 as a reliable semiconductor source for compact, high-power THz radiation. The inherently strong third-order nonlinearity in its QC-gain medium allows for spontaneous frequency comb formation as a result of spatial hole burning induced by Fabry-Perot cavities and four-wave mixing, which synchronizes the dispersed cavity modes. It was noticed that the self-generated combs are naturally frequency-modulated with quasi-continuous power output, whereas amplitude-modulated combs, i.e., mode-locking, are considered challenging in THz QCLs because of the inherent fast gain recovery time. One effective method to trigger active mode-locking is RF injection locking. It involves injecting RF current modulation into the QC-device at a frequency that is close to the cavity round-trip frequency. This locks the spacing between adjacent lasing modes, and pulses with a duration of 4-5 ps have been reported. In recent years, the study of frequency comb/mode-locking in THz QCLs has raised increasing interest because of its potential for a number of applications, including astronomy, biomedicine, fast spectroscopy, non-invasive imaging, and non-destructive evaluation. So far, research has concentrated on ridge-waveguide and ring QCLs. On the other hand, THz quantum-cascade vertical-external-cavity surface-emitting-laser (QC-VECSEL) was introduced in 2015 as a novel external cavity configuration of THz QCLs.The key concept of THz QC-VECSEL is to engineer its gain chip into a millimeter-scale reflectarray metasurface for free-space THz radiation and further incorporation into a resonant laser cavity as an active reflector. This enables watt-level output power with near-Gaussian distributed beam quality; versatile functionality may be incorporated into the amplifying metasurface; and broadband frequency tunability is provided by the VECSEL architecture. Despite the fact that VECSELs are widely used for mode-locking at near-infrared and optical frequencies, THz QC-VECSELs have not yet been exploited in frequency comb and mode-locking applications. In this thesis, we report for the first time the techniques utilized to achieve frequency comb/mode-locking operations in THz QC-VECSELs. Both the metasurface design and VECSEL cavity geometry are optimized for this purpose. The double-patch metasurface design is considered optimal for broadband frequency response and low dispersion, and a well-designed RF package is needed for efficient RF signal injection and extraction. On the other hand, an off-axis parabolic (OAP) mirror is introduced to build a V-shaped intra-cryostat focusing VECSEL cavity. This OAP-focusing cavity design eliminates most of the intra-cavity diffraction losses and, therefore, enables lasing in an ultra-long external cavity using a small-sized metasurface that supports continuous wave (CW) biasing. It is highly suited for frequency comb/mode-locking applications as the cavity round-trip frequency is lowered to a typical value of 3-5 GHz. In contrast to ridge-waveguide or ring QCLs, self-generated frequency combs have not been observed in THz QC-VECSELs --- in fact, they prefer to lase in a single-mode regime primarily due to a lack of spatial hole burning.To promote multimode operation in THz QC-VECSELs, we present a technique based on a specific combination of output coupler thickness and external cavity length. Through Vernier selection and reflectance compensation in a cascaded Fabry-Perot cavity, we are able to perform simultaneous nine modes lasing with a free-spectral range (FSR) of ~21 GHz. The number of lasing modes that can be generated using this method is limited by the maximum available output coupler thickness. A more effective way to promote multimoding, as well as possible frequency comb or even mode-locking operations, is through RF injection locking.The successful demonstration of RF injection locking in THz QC-VECSELs for the first time is the main focus of this thesis. Lasing spectral broadening has been observed under strong RF modulation, with a maximum bandwidth of around 100-300 GHz. An intermodal beat-note is produced as a result of beating between each of the two lasing modes. It is locked to the RF injection signal as the injection frequency is tuned around the cavity round-trip frequency. This suggests that the lasing modes are equally spaced, which is a prerequisite of frequency comb/mode-locking. Several impacting factors, including metasurface design, external cavity length, and optical feedback, are experimentally investigated in the RF-injection locked QC-VECSELs, which may help control and tune the laser states. THz QC-VECSEL is consequently considered to be a superior platform that enables a more thorough investigation of the fundamental physics of mode-locking/frequency comb operation in QCL systems. Our research on mode-locked THz QC-VECSELs opens the way for future development of semiconductor lasers operating in the 2-5 THz region that produce picosecond-scale pulses.

Author : Tianyi Zeng
Publisher :
Page : 105 pages
File Size : 10,97 MB
Release : 2017
Category :
ISBN :

GET BOOK

Ever since the invention of quantum cascade laser (QCL), the performance and the flexibility in design has made it a desirable source for a wide range of applications, such as trace-chemical sensing, health monitoring, frequency metrology, noninvasive imgaing and infrared countermeasures. The LWIR region (or mid-infrared region), roughly ranging from 2-20 [mu]m, is of particular importance to spectroscopy applications, since many molecular species have their strongest rotational-vibrational absorption bands in that area. Infrared laser spectroscopy began about 40 years ago and has been using a variety of different tunable laser-based sources, particularly lead salt diodes, color center lasers, difference frequency generation and optical parametric oscillators. The large tunabilitiy in the design (lasing frequency, tunability, power, material system, etc.) and the compactness in fabrication and packaging has made QCL an ideal source for laser-based spectroscopy. Traditional spectroscopy systems suffer from problems like large physical dimensions, long data-processing times and spectral resolution restrictions. Therefore the development of a simple, robust, compact and inexpensive optical source/system like QCL frequency combs can largely benefit spectroscopy systems. In the past few years, QCLs have proven to be able to form comb radiation in both LWIR and THz regions. And dual comb spectroscopy has been demonstrated using QCL frequency combs with very short acquisition time ([mu]s). The development of a broadband, high power, narrow linewidth and stable LWIR frequency comb based on quantum cascade laser is the key to realizing such broadband ultrafast spectrometer in the mid-infrared range. This thesis explores the design, fabrication and characterization techniques towards the development of LWIR QCL frequency comb devices for spectroscopic purposes. A complete wet etch epi-up fabrication process is reported, with preliminary results on the dry-etch technique to incorporate dispersion compensation strucutre and epi-down fabricaiton for high power CW mode QCL device. Formation of comb(-like) regime has been observed in two devices, with the Gires-Tournois Interferometer (GTI) mirror providing dispersion from the rear facet. In order to improve the comb performance of these devices, dispersion of the device is measured to provide essential information for the design of chirped top cladding for dispersion compensation. This thesis provides an important step towards the realization of a room temperature, broadband, CW mode LWIR QCL frequency comb device for spectroscopic purposes.

Author :
Publisher :
Page : 4 pages
File Size : 35,25 MB
Release : 2016
Category :
ISBN :

GET BOOK

The terahertz region is of great importance for spectroscopy since many molecules have absorption fingerprints there. Frequency combs based on terahertz quantum cascade lasers feature broadband coverage and high output powers in a compact package, making them an attractive option for broadband spectroscopy. Here, we demonstrate the first multiheterodyne spectroscopy using two terahertz quantum cascade laser combs. Over a spectral range of 250 GHz, we achieve average signal-to-noise ratios of 34 dB using cryogenic detectors and 24 dB using room-temperature detectors, all in just 100 [mu]s. As a proof of principle, we use these combs to measure the broadband transmission spectrum of etalon samples and show that, with proper signal processing, it is possible to extend the multiheterodyne spectroscopy to quantum cascade laser combs operating in pulsed mode. As a result, this greatly expands the range of quantum cascade lasers that could be suitable for these techniques and allows for the creation of completely solid-state terahertz laser spectrometers.

Author : Chun Wang Ivan Chan
Publisher :
Page : 251 pages
File Size : 41,82 MB
Release : 2015
Category :
ISBN :

GET BOOK

Terahertz Quantum Cascade Lasers (THz QCLs) are arguably the most promising technology today for the compact, efficient generation of THz radiation. Their main limitation is that they require cryogenic cooling, which dominates their ownership cost. Therefore, achieving room-temperature operation is essential for the widespread adoption of THz QCLs. This thesis analyzes the limitations of THz QCL maximum lasing temperature (Tmax) and proposes solutions. THz QCL Tmax is hypothesized to be limited by a fundamental trade-off between gain oscillator strength ful and upper-level lifetime [Tau]. This so-called "ful[Tau] tradeoff" is shown to explain the failure of designs which target [Tau] alone. A solution is proposed in the form of highly diagonal (low ful) active region design coupled with increased doping. Experimental results indicate the strategy to be promising, but heavily doped designs are shown to suffer band-bending effects which may deteriorate performance. In order to treat these band-bending effects, which are typically neglected in previous THz QCL designs, a fast transport simulation tool is developed. Scattering integrals are simplified using the assumption of thermalized sub bands. Results comparable to ensemble Monte Carlo are achieved at a fraction of the computational expense. Carrier leakages to continuum states are also investigated, although they are found to have little effect. Other work in this thesis includes the optimization of double-metal THz waveguides to enable Tmax ~ 200 K, a current world record. Furthermore, laser designs to investigate the leakages of carriers to high-energy subbands and continuum states were fabricated and tested; such parasitic leakages are suggested to be small. Finally, the design of gain media for applications is examined, notably the development of 4.7 THz gain media for OI line detection in astrophysics, and the development of broadband heterogeneous gain media for THz comb generation.