[PDF] Plasmonic Generation Of Attosecond Pulses And Attosecond Imaging Of Surface Plasmons eBook

Author : Phillip Michael Nagel
Publisher :
Page : 190 pages
File Size : 23,12 MB
Release : 2011
Category :
ISBN :

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Surface plasmon resonances (SPRs), collective oscillations of quasi-free electrons in metals, can produce strong electric field enhancements at the surface of nanoparticles. These oscillations typically occur at optical frequencies (thus having a period on the order of one to a few femtoseconds) and only remain coherent for a few to tens of femtoseconds. Because of their increasing importance in various applications, it is important to understand SPRs at a fundamental level. The ultrafast nature of the processes involved with SPRs make time-resolved spectroscopy an important tool for probing their dynamics. Recently developed light sources capable of producing isolated attosecond (10-̂18 s) pulses of light can provide snapshots of electron dynamics on a sub-femtosecond timescale. Fewer than a dozen laboratories in the world currently have the ability to produce such light pulses. In this dissertation I discuss the development and construction of an experimental apparatus capable of producing and utilizing isolated attosecond pulses to study condensed matter, including surface plasmon dynamics. The ultimate goal of the experiments presented here is to laser-excite plasmonic resonances in metallic nanostructures and to detect the field enhancement at the surface of the nanostructures by measuring photoelectron spectra. In the first experiment presented, electron photoemission from lithographically prepared gold nanopillars using nominally few-cycle, 800 nm laser pulses is described. Electron kinetic energies are observed that are higher by up to tens of eV compared to photoemission from a flat gold surface at the same laser intensities. A classical electron acceleration model consisting of multiphoton ionization followed by field acceleration qualitatively reproduces the electron kinetic energy data and suggests average enhanced electric fields due to the nanopillars that are between 25 and 39 times greater than the experimentally used laser fields. In the second experiment presented, attosecond streaking from a W(110) single crystal and from an amorphous Cr thin film is demonstrated. In addition, a novel concept for SPR enhanced attosecond streaking is proposed and evaluated with the aid of a numerical model.

Author : Peter Hommelhoff
Publisher : John Wiley & Sons
Page : 392 pages
File Size : 31,3 MB
Release : 2015-03-09
Category : Science
ISBN : 3527411712

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Die Autoren geben einen tiefen wie auch umfassenden Überblick über die aktuelle Forschung im Bereich der Attosekunden-Nanophysik, d.h. einem Gebiet der nanoskaligen Festkörpersysteme und der natürlichen Zeitskala von Elektronenbewegungen.

Author : Stefan Alexander Maier
Publisher : Springer Science & Business Media
Page : 234 pages
File Size : 14,7 MB
Release : 2007-05-16
Category : Technology & Engineering
ISBN : 0387378251

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Considered a major field of photonics, plasmonics offers the potential to confine and guide light below the diffraction limit and promises a new generation of highly miniaturized photonic devices. This book combines a comprehensive introduction with an extensive overview of the current state of the art. Coverage includes plasmon waveguides, cavities for field-enhancement, nonlinear processes and the emerging field of active plasmonics studying interactions of surface plasmons with active media.

Author : Stefan Enoch
Publisher : Springer
Page : 331 pages
File Size : 20,13 MB
Release : 2012-06-30
Category : Science
ISBN : 364228079X

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This book deals with all aspects of plasmonics, basics, applications and advanced developments. Plasmonics is an emerging field of research dedicated to the resonant interaction of light with metals. The light/matter interaction is strongly enhanced at a nanometer scale which sparks a keen interest of a wide scientific community and offers promising applications in pharmacology, solar energy, nanocircuitry or also light sources. The major breakthroughs of this field of research originate from the recent advances in nanotechnology, imaging and numerical modelling. The book is divided into three main parts: extended surface plasmons polaritons propagating on metallic surfaces, surface plasmons localized on metallic particles, imaging and nanofabrication techniques. The reader will find in the book: Principles and recent advances of plasmonics, a complete description of the physics of surface plasmons, a historical survey with emphasize on the emblematic topic of Wood's anomaly, an overview of modern applications of molecular plasmonics and an extensive description of imaging and fabrications techniques.

Author : Peng Yu
Publisher : Springer Nature
Page : 348 pages
File Size : 41,76 MB
Release : 2022-03-01
Category : Science
ISBN : 303087544X

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This book highlights cutting-edge research in surface plasmons, discussing the different types and providing a comprehensive overview of their applications. Surface plasmons (SPs) receive special attention in nanoscience and nanotechnology due to their unique optical, electrical, magnetic, and catalytic properties when operating at the nanoscale. The excitation of SPs in metal nanostructures enables the manipulation of light beyond the diffraction limit, which can be utilized for enhancing and tailoring light-matter interactions and developing ultra-compact high-performance nanophotonic devices for various applications. With clear and understandable illustrations, tables, and descriptions, this book provides physicists, materials scientists, chemists, engineers, and their students with a fundamental understanding of surface plasmons and device applications as a basis for future developments.

Author : Olga Lozan
Publisher :
Page : 0 pages
File Size : 25,77 MB
Release : 2015
Category :
ISBN :

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In this work we explored the ultrafast dynamics of photo-excited hot electrons in plasmonic structures. The particular interest of this field resides on the fact surface plasmons (SP), because of their unrivaled temporal and spatial characteristics, provide a technological route for ultrafast information processes at the nanoscale. In this context, this manuscript provides a comprehension and the harnessing of one of the major limitation of the SP-based technologies : absorption losses by Joule heating. We exploit the fact that the mechanism of plasmon absorption in metals is followed by generation of hot electrons at femtosecond time scale, thus losses can be seen as a plasmon-to-hot-electron energy conversion. This energy conversion is measured with femtosecond pump-probe technique. Femtosecond SP pulses are launched and probed over hundred femtoseconds through the permittivity variations induced by the hot-electron gas and which accompany the SP propagation. The measured electron temperature profile is therefore an image of plasmon power density distribution (absorption) not broadened spatially and temporally by energy carrier diffusion. As an important result we demonstrated the capability to link the electronic temperature measurement to the plasmonic absorption, revealing an anomalous light absorption for a sub- slit surroundings, in quantitative agreement with predictions of the power density distribution. In a second part we studied plasmon losses and their characteristics when they propagate on semi-infinite metal film. We determined the electronic thermal wave velocity and damping. In the last part we used a focusing taper-structure to adiabatically guide and focus the plasmon at the apex. Was demonstrated the generation of a nanoscale hot spot and put in evidence a delayed electron heating at the taper apex. Perspectives and the remaining open questions are also discussed.

Author : Markus Kitzler
Publisher : Springer
Page : 385 pages
File Size : 22,64 MB
Release : 2015-07-24
Category : Science
ISBN : 3319201735

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This book documents the recent vivid developments in the research field of ultrashort intense light pulses for probing and controlling ultrafast dynamics. The recent fascinating results in studying and controlling ultrafast dynamics in ever more complicated systems such as (bio-)molecules and structures of meso- to macroscopic sizes on ever shorter time-scales are presented. The book is written by some of the most eminent experimental and theoretical experts in the field. It covers the new groundbreaking research directions that were opened by the availability of new light sources such as fully controlled intense laser fields with durations down to a single oscillation cycle, short-wavelength laser-driven attosecond pulses and intense X-ray pulses from the upcoming free electron lasers. These light sources allowed the investigation of dynamics in atoms, molecules, clusters, on surfaces and very recently also in nanostructures and solids in new regimes of parameters which, in turn, led to the identification of completely new dynamics and methods for controlling it. Example topics covered by this book include the study of ultrafast processes in large molecules using attosecond pulses, control of ultrafast electron dynamics in solids with shaped femtosecond laser pulses, light-driven ultrafast plasmonic processes on surfaces and in nanostructures as well as research on atomic and molecular systems under intense X-ray radiation. This book is equally helpful for people who would like to step into this field (e.g. young researchers), for whom it provides a broad introduction, as well as for already experienced researchers who may enjoy the exhaustive discussion that covers the research on essentially all currently studied objects and with all available ultrafast pulse sources.

Author : Thomas Schultz
Publisher : John Wiley & Sons
Page : 624 pages
File Size : 31,11 MB
Release : 2013-11-13
Category : Science
ISBN : 3527677658

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This book provides fundamental knowledge in the fields of attosecond science and free electron lasers, based on the insight that the further development of both disciplines can greatly benefit from mutual exposure and interaction between the two communities. With respect to the interaction of high intensity lasers with matter, it covers ultrafast lasers, high-harmonic generation, attosecond pulse generation and characterization. Other chapters review strong-field physics, free electron lasers and experimental instrumentation. Written in an easy accessible style, the book is aimed at graduate and postgraduate students so as to support the scientific training of early stage researchers in this emerging field. Special emphasis is placed on the practical approach of building experiments, allowing young researchers to develop a wide range of scientific skills in order to accelerate the development of spectroscopic techniques and their implementation in scientific experiments. The editors are managers of a research network devoted to the education of young scientists, and this book idea is based on a summer school organized by the ATTOFEL network.

Author : Zhaowei Liu
Publisher : CRC Press
Page : 278 pages
File Size : 38,62 MB
Release : 2017-06-26
Category : Science
ISBN : 135179731X

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Plasmonics is an emerging field mainly developed within the past two decades. Due to its unique capabilities to manipulate light at deep subwavelength scales, plasmonics has been commonly treated as the most important part of nanophotonics. Plasmonic-assisted optical microscopy techniques, especially super-resolution microscopy, have shown tremendous potential and attracted much attention. This book aims to collect cutting-edge studies in various optical imaging technologies with advanced performances that are enabled or enhanced by plasmonics. The basic working principles, development details, and potential future direction and perspectives are discussed. Edited by Zhaowei Liu, a prominent researcher in the field of super-resolution microscopy, this book will be an excellent reference for anyone in the field of nanophotonics, plasmonics, and optical microscopy.