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Author : Michael F. Hochella Publisher : Walter de Gruyter GmbH & Co KG Page : 620 pages File Size : 45,96 MB Release : 2018-12-17 Category : Science ISBN : 1501509136
Volume 23 of Reviews in Mineralogy and accompanying MSA short course covers chemical reactions that take place at mineral-water interfaces. We believe that this book describes most of the important concepts and contributions that have driven mineral-water interface geochemistry to its present state. We begin in Chapter 1 with examples of the global importance of mineral-water interface reactions and a brief review of the contents of the entire book. Thereafter, we have divided the book into four sections, including atomistic approaches (Chapters 2- 3), adsorption (Chapters 4-8), precipitation and dissolution (Chapters 9-11), and oxidation-reduction reactions (Chapters 11-14).
Provides an introduction to the chemistry of the solid-water interface, progressing from the simple to more complex and applied. Discusses the important interfaces in natural systems, especially geochemistry, in natural waters, soils and sediments. The processes occurring at mineral-water, particle-water and organism-water interfaces play critical roles in regulating the composition and ecology of oceans and fresh waters, the development of soils and plant nutrient's supply, preserving the integrity of water repositories and in such applications as water technology and corrosion science.
Clearly explains how to more effectively decipher and predict contaminant fate in the environment by combining kinetic methods and molecular-scale spectroscopic and microscopic techniques to analyze mineral/water interfacial reactions in situ. The book begins with a broad overview, then continues with three sections written by internationally known expert. The first deals specifically with spectroscopic/microscopic techniques that can be used in combination with macroscopic approaches to glean mechanistic information on mineral/water reactions and processes. The second section emphasizes computer models that are used to elucidate surface mediated reaction mechanisms. The remainder of the volume is organized around reaction type, including sorption/desorption of inorganic species, sorption/desorption of organic species, precipitation/dissolution processes, heterogeneous electron transfer reactions, photochemically driven reactions, and microbially mediated reactions. Mineral-Water Interfacial Reactions will be a valuable resource for environmental scientists, geochemists, soil chemists, microbiologists, and marine engineers who need to be familiar with the most current and effective methods for testing and controlling the mobility, speciation, and bioavailability of contaminants in the environment.
The project emphasis at WSU is on the understanding of the principal influences on surface chemistry, morphology, and kinetics of reactions of minerals in aqueous solutions. This emphasis, in the last project period has guided our efforts to the study of morphological relaxation in response to solution perturbations as well as to develop a methodology for creating on-demand etch pits for the purposes of generating specific step orientations on calcite surfaces. In the response of any mineral-water interface to changes in environmental conditions, dissolution and mineralization rates undergo rapid changes because the reaction rates at step edges are governed directly by these conditions. Our previous investigations of mineral dissolution have revealed that the topographic relaxation time under near equilibrium conditions can be much longer than the characteristic times of experimental investigations. The investigations described below are directed towards evaluating the effects of sample history, miscut and pretreatment on the observed dissolution behavior of our target mineral-water interface systems. In addition, we have developed a simple method for generating on-demand etch pits for the purposes of studying kinetically unstable step orientations.
Author : Eric H. Oelkers Publisher : Walter de Gruyter GmbH & Co KG Page : 588 pages File Size : 22,15 MB Release : 2018-12-17 Category : Science ISBN : 1501508466
Volume 70 of Reviews in Mineralogy and Geochemistry represents an extensive review of the material presented by the invited speakers at a short course on Thermodynamics and Kinetics of Water-Rock Interaction held prior to the 19th annual V. M. Goldschmidt Conference in Davos, Switzerland (June 19-21, 2009). Contents: Thermodynamic Databases for Water-Rock Interaction Thermodynamics of Solid Solution-Aqueous Solution Systems Mineral Replacement Reactions Thermodynamic Concepts in Modeling Sorption at the Mineral-Water Interface Surface Complexation Modeling: Mineral Fluid Equilbria at the Molecular Scale The Link Between Mineral Dissolution/Precipitation Kinetics and Solution Chemistry Organics in Water-Rock Interactions Mineral Precipitation Kinetics Towards an Integrated Model of Weathering, Climate, and Biospheric Processes Approaches to Modeling Weathered Regolith Fluid-Rock Interaction: A Reactive Transport Approach Geochemical Modeling of Reaction Paths and Geochemical Reaction Networks
Geochemical kinetics as a topic is now of importance to a wide range of geochemists in academia, industry, and government, and all geochemists need a rudimentary knowledge of the field. This book summarizes the fundamentals of geochemical kinetics with examples drawn especially from mineral dissolution and precipitation. It also encompasses discussion of high temperature processes and global geochemical cycle modeling. Analysis of textures of rocks, sediments, and mineral surfaces are incorporated throughout and provide a sub-theme of the book.
In Europe, ca. 1900 "mineral water" brandsare officially registered and bottled for drinking. Bottled waters isgroundwater and is in large parts of the continent rapidly developing into themain supply of drinking water for the general population.This book is the first state of the art overview of the chemistry ofgroundwaters from 40 European countries from Portugal to Russia, measured on1785 bottled water samples, equivalent to 1189 distinct bottled water brandsfrom 1247 wells in 884 locations plus an additional 500 tap water samplesacquired in 2008 by the network of EuroGeoSurveys experts all across Europe.In contrast to previously available compilations, all chemical data (containedon the enclosed CD) were measured in a single laboratory, under strict qualitycontrol with high internal and external reproducibility, affording a singlehigh quality, internally consistent dataset. More than 70 parameters weredetermined on every sample using state of the art analytical techniques withultra low detection limits (ICPMS, ICPOES, IC) at a single hydrochemical labfacility. Because of the wide geographical distributionof the water sources across 40 European countries, the bottled mineral,drinking and tap waters characterized herein may be used for obtaining a firstestimate of "ground- water geochemistry" at the scale of the EuropeanContinent, previously unavailable in this completeness, quality and coverage.The data published here allow for the first time to present a comprehensiveinternally consistent, overview of the natural distribution and variation ofthe determined chemical elements and additional state parameters of groundwaterat the European scale. Most elements show a very widerange, usually 3 to 4 but up to 7 orders of magnitude, of natural variation of their concentration. Data are interpreted in terms of their origin, considering hydrochemical parameters, such as the influence of soil, vegetation cover and mixing with deep waters, as well as other factors (bottling effects, leaching from bottles). A chapter is devoted to comparing the results from the bottled waters with those of European tap waters and previously published datasets. The authors also provide an overview of the legal framework, that any bottled water sold in the European Union must comply with. It provides a comprehensive compilation of current drinking water action levels in European countries, limiting values of the European Drinking/Mineral/Natural Mineral Water directives (1998/83/EC, 2003/40/EC, 2009/54/EC) and legislation in effect in 26 individual European Countries, and for comparison those of the FAO and in effect in the US (EPA, maximum contaminant levels [MCA]). The accompanying CD contains the extensive data sets, sample data (of 1189 different brands) and two previously published European water chemistry data sets.
30% discount for members of The Mineralogical Society of Britain and Ireland This text summarises the state-of-the-art in the study of mineral surfaces and some of the key applications of surface science in mineralogy and mineral chemistry. Each chapter covers a particular aspect of the subject and is written by an expert who raises the key issues involved for those requiring an introduction to the subject, whilst highlighting most recent developments. Advanced undergraduates, postgraduates and researchers alike will find this essential reading as it is the first book to review the fast developing field of mineral surfaces.