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Materials Interaction with Femtosecond Lasers

Author : Bernd Bauerhenne
Publisher :
Page : 0 pages
File Size : 47,39 MB
Release : 2021
Category :
ISBN : 9783030851361

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This book presents a unified view of the response of materials as a result of femtosecond laser excitation, introducing a general theory that captures both ultrashort-time non-thermal and long-time thermal phenomena. It includes a novel method for performing ultra-large-scale molecular dynamics simulations extending into experimental and technological spatial dimensions with ab-initio precision. For this, it introduces a new class of interatomic potentials, constructed from ab-initio data with the help of a self-learning algorithm, and verified by direct comparison with experiments in two different materials - the semiconductor silicon and the semimetal antimony. In addition to a detailed description of the new concepts introduced, as well as giving a timely review of ultrafast phenomena, the book provides a rigorous introduction to the field of laser-matter interaction and ab-initio description of solids, delivering a complete and self-contained examination of the topic from the very first principles. It explains, step by step from the basic physical principles, the underlying concepts in quantum mechanics, solid-state physics, thermodynamics, statistical mechanics, and electrodynamics, introducing all necessary mathematical theorems as well as their proofs. A collection of appendices provide the reader with an appropriate review of many fundamental mathematical concepts, as well as important analytical and numerical parameters used in the simulations.

Femtosecond Laser-Matter Interaction

Author : Eugene G. Gamaly
Publisher : CRC Press
Page : 370 pages
File Size : 13,30 MB
Release : 2011-10-06
Category : Science
ISBN : 9814241814

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This is the first comprehensive treatment of the interaction of femtosecond laser pulses with solids at nonrelativistic intensity. It connects phenomena from the subtle atomic motion on the nanoscale to the generation of extreme pressure and temperature in the interaction zone confined inside a solid. The femtosecond laser-matter interaction has already found numerous applications in industry, medicine, and materials science. However, there is no consensus on the interpretation of related phenomena. With mathematics kept to a minimum, this is a highly engaging and readable treatment for students and researchers in science and engineering. The book avoids complex mathematical formulae, and hence the content is accessible to nontechnical readers. Useful summaries after each chapter provide compressed information for quick estimates of major parameters in planned or performed experiments. The book connects the basic physics of femtosecond laser-solid interactions to a broad range of applications. Throught the text, basic assumptions are derived from the first principles, and new results and ideas are presented. From such analyses, a qualitative and predictive framework for the field emerges, the impact of which on applications is also discussed.

Coherent Optical Interactions in Semiconductors

Author : R.T. Phillips
Publisher : Springer Science & Business Media
Page : 362 pages
File Size : 41,24 MB
Release : 2013-06-29
Category : Science
ISBN : 1475797486

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The NATO Advanced Research Workshop on Coherent Optical Processes in Semiconductors was held in Cambridge, England on August 11-14,1993. The idea of holding this Workshop grew from the recent upsurge in activity on coherent transient effects in semiconductors. The development of this field reflects advances in both light sources and the quality of semiconductor structures, such that tunable optical pulses are now routinely available whose duration is shorter than the dephasing time for excitonic states in quantum wells. It was therefore no surprise to the organisers that as the programme developed, there emerged a heavy emphasis on time-resolved four-wave mixing, particularly in quantum wells. Nevertheless, other issues concerned with coherent effects ensured that several papers on related problems contributed some variety. The topics discussed at the workshop centred on what is a rather new field of study, and benefited enormously by having participants representing many of the principal groups working in this area. Several themes emerged through the invited contributions at the Workshop. One important development has been the careful examination of the two-level model of excitonic effects; a model which has been remarkably successful despite the expected complexities arising from the semiconductor band structure. Indeed, modest extensions to the two level model have been able to offer a useful account for some of the complicated polarisation dependence of four-wave mixing signals from GaAs quantum wells. This work clearly is leading to an improved understanding of excitons in confined systems.

Mid-infrared Strong-field Laser Interactions with Nanoclusters and Semiconductors

Author : Zhou Wang (Ph. D. in physics)
Publisher :
Page : 168 pages
File Size : 25,48 MB
Release : 2018
Category : Physics
ISBN :

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In the interaction of intense infrared lasers with atoms/molecules, an ionized election is accelerated by the laser field, and revisits the parent ion. High energy electrons are generated after rescattering with the ion, or alternatively, harmonic photons are emitted as attosecond bursts after electron-ion recombination. However, the validity of the picture requires verification in condensed-phase targets. This study discusses the behavior of nanoclusters and semiconductors under intense femtosecond laser fields. In the laser interaction with nanoclusters, photoelectron and charged ion emission are investigated at various driving laser wavelengths. In the study of photoelectrons, we show that the laser-field-driven rescattering picture is still valid in nanoclusters after adaptions. With the help of tunable laser wavelength, we observe an extension of cutoff energy and discover its universal scaling with the cluster size and driving wavelength. On the other hand, a wavelength-dependent ion emission is observed, which sheds light on the underlying cluster dynamics. In addition, the ion emission is managed to be controlled with a tailored pulse. In the laser interaction with semiconductors, the high harmonic photon emission driven by mid-infrared lasers are measured, which comes from distinct mechanisms from atoms/molecules. The roles of photocarrier density and driving wavelength are explored, which not only convey the information of underlying mechanisms, but also suggest approaches to optimize the harmonic generation conditions for future table-top attosecond burst generation. Moreover, a two-color beam is applied to drive the harmonic emission from solids and an enhanced frequency-upconversion efficiency is observed.

Femtosecond Laser-Matter Interactions

Author : Eugene G. Gamaly
Publisher : CRC Press
Page : 294 pages
File Size : 32,14 MB
Release : 2022-01-31
Category : Technology & Engineering
ISBN : 1000522830

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This book describes the ultra-short laser–matter interactions from the subtle atomic motion to the generation of extreme pressures inside the bulk of a transparent crystal. It is the successor to Femtosecond Laser–Matter Interactions: Theory, Experiment and Applications (2011). Explanation and experimental verification of the exceptional technique for the phase transformations under high pressure are in the core of the book. The novel phase formation occurs along the unique solid-plasmasolid transformation path: the memory of the initial state is lost after conversion to plasma. New phase forms from chaos during the cooling to the ambient. The pressure-affected material remains detained inside a pristine crystal at the laboratory tabletop. Unique super-dense aluminium and new phases of silicon were created by the confined micro-explosions. The text also describes the recent studies that used the quasi-non-diffracting Bessel beams. The applications comprise the new high-pressure material formation and micromachining. The book is an appealing source for readers interested in the cutting-edge research exploring extreme conditions and creating nanostructures at the laboratory tabletop.

Femtosecond Laser Pulses

Author : Claude Rulliere
Publisher : Springer Science & Business Media
Page : 438 pages
File Size : 13,61 MB
Release : 2007-05-27
Category : Science
ISBN : 0387266747

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This smooth introduction for advanced undergraduates starts with the fundamentals of lasers and pulsed optics. Thus prepared, the student is introduced to short and ultrashort laser pulses, and learns how to generate, manipulate, and measure them. Spectroscopic implications are also discussed. The second edition has been completely revised and includes two new chapters on some of the most promising and fast-developing applications in ultrafast phenomena: coherent control and attosecond pulses.

Femtosecond Laser-Matter Interaction

Author : Eugene G. Gamaly
Publisher : CRC Press
Page : 350 pages
File Size : 33,39 MB
Release : 2011-10-06
Category : Science
ISBN : 9814267805

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This is the first comprehensive treatment of the interaction of femtosecond laser pulses with solids at nonrelativistic intensity. It connects phenomena from the subtle atomic motion on the nanoscale to the generation of extreme pressure and temperature in the interaction zone confined inside a solid. The femtosecond laser-matter interaction has al

Femtosecond Technology

Author : T. Kamiya
Publisher : Springer Science & Business Media
Page : 449 pages
File Size : 28,8 MB
Release : 2012-12-06
Category : Science
ISBN : 3642584691

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Recent rapid advances in femtosecond technology have had a great impact on their industrial applications such as: ultrafast optoelectronic devices and optical telecommunication systems, ultrashort-pulse lasers and measurement systems, and the development of novel materials for ultrafast functions. In this book, a wealth of knowledge covering requirements in applications details of recent achievements in important technical areas is presented by world-prominent authors in a concise, systematic form. As a whole, this is the first comprehensive book on the emerging field of femtosecond technology.