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One of the most important applications for Terahertz (THz) quantum cascade (QC) lasers is to provide compact and powerful frequency-stabilized solid-state sources as local oscillators in heterodyne receivers for astronomical studies. The first part of the thesis is dedicated to the device cavity design, fabrication and characterization of the microstrip antenna coupled third-order distributed feedback QC lasers aimed for 2.060 THz atomic oxygen line. THz travelling-wave QC amplifiers are highly desired to achieve broadband amplification of THz radiation in free space. The second part of the thesis focuses on the development of 4.3 THz travelling-wave QC amplifier by monolithically integrating horn antennas and attaching silicon lenses at the metal-metal waveguide facets.
Terahertz Quantum Cascade Lasers (THz QCLs) are arguably the most promising technology today for the compact, efficient generation of THz radiation. Their main limitation is that they require cryogenic cooling, which dominates their ownership cost. Therefore, achieving room-temperature operation is essential for the widespread adoption of THz QCLs. This thesis analyzes the limitations of THz QCL maximum lasing temperature (Tmax) and proposes solutions. THz QCL Tmax is hypothesized to be limited by a fundamental trade-off between gain oscillator strength ful and upper-level lifetime [Tau]. This so-called "ful[Tau] tradeoff" is shown to explain the failure of designs which target [Tau] alone. A solution is proposed in the form of highly diagonal (low ful) active region design coupled with increased doping. Experimental results indicate the strategy to be promising, but heavily doped designs are shown to suffer band-bending effects which may deteriorate performance. In order to treat these band-bending effects, which are typically neglected in previous THz QCL designs, a fast transport simulation tool is developed. Scattering integrals are simplified using the assumption of thermalized sub bands. Results comparable to ensemble Monte Carlo are achieved at a fraction of the computational expense. Carrier leakages to continuum states are also investigated, although they are found to have little effect. Other work in this thesis includes the optimization of double-metal THz waveguides to enable Tmax ~ 200 K, a current world record. Furthermore, laser designs to investigate the leakages of carriers to high-energy subbands and continuum states were fabricated and tested; such parasitic leakages are suggested to be small. Finally, the design of gain media for applications is examined, notably the development of 4.7 THz gain media for OI line detection in astrophysics, and the development of broadband heterogeneous gain media for THz comb generation.
Learn how the rapidly expanding area of mid-infrared and terahertz photonics has been revolutionized in this comprehensive overview. State-of-the-art practical applications are supported by real-life examples and expert guidance. Also featuring fundamental theory enabling you to improve performance of both existing and future devices.
Quantum cascade lasers are unipolar semiconductor lasers based on intersubband transitions in quantum wells. They have shown laser operation from above 100 THz down to the terahertz region and are promising sources for the terahertz region (0.3-10 THz) which is lacking of efficient narrowband radiation sources. A low frequency quantum cascade laser design is developed that faces the emerging challenges when the photon energy approaches the broadening of the energy levels. A record lowest operation frequency of 1.2 THz is demonstrated. A hybrid laser-oscillator for the terahertz is developed in the second part of this work, consisting of an optical gain medium and an electronic resonator. The resonator is an inductor-capacitor resonant circuit. The so called circuit based laser has the property of being a deep sub-wavelength sized microcavity laser. The effective mode volume is among the smallest for electrically pumped lasers. The circuit based resonator in combination with an active region could lead to a class of new devices to generate and manipulate terahertz radiation that exploit cavity quantum electrodynamic effects.
Terahertz (THz) quantum-cascade lasers (QCLs) are an emerging semiconductor source of compact, high-power THz radiation. Though first realized more than 15 years ago, THz QCLs continue to suffer from poor beam quality and outcoupling efficiency due to the subwavelength nature of the semiconductor ridge-waveguides typically used. In this thesis, a new technique is discussed for obtaining high power and good beam quality from THz QCLs, the THz quantum-cascade external cavity surface emitting laser (QC-VECSEL). The concept of the QC-VECSEL is to use THz QC-gain material to design a millimeter-scale reflective amplifying surface, or metasurface, for free space THz waves and incorporate it into a free-space THz resonant cavity to provide feedback to the amplification and form a laser. In this manner, the beam shape is determined by the external cavity, which supports fundamental Gaussian solutions. Further, the metasurface itself is composed of a subwavelength array (to prevent diffraction) of surface-coupled QC-elements whose properties, such as phase and polarization response, can be engineered on a unit cell basis allowing for a variety of unique experiments. The power output power of the QC-VECSEL can be scaled by either increasing the size of the metasurface, or increasing the density (or fill factor) of QC-elements across the surface. In this work, large area metasurfaces with high fill-factor have been studied and demonstrated up to 1.35 W of peak output power for a QC-VECSEL operating at 3.4 THz at a heat sink temperature of 4 K. A peak wall-plug efficiency of ~2% is demonstrated, but observation of self lasing from the metasurface at high bias (when no external cavity is provided) in combination with a simultaneous roll-off in VECSEL output power suggests even higher efficiency can be achieved with improved suppression of self-lasing modes. The output beam is well fit to a Gaussian distribution with a 4 degree full-width half-maximum divergence angle. In addition to power and beam quality, the QC-VECSEL opens the door to many interesting and unique studies via engineering of the metasurface properties and external cavity. Much of this thesis describes frequency tuning of QC-VECSELs based on broadband metasurfaces by varying the length of the external cavity. By making the external cavity extremely short (comparable to the operating wavelength), we are able to push all other external cavity modes outside of the gain bandwidth of the metasurface and demonstrate more than 20% fractional single-mode tuning around a center operating frequency of 3.5 THz. Because there are almost no diffraction losses at such a short cavity, the size of the metasurface could be reduced, allowing for continuous wave lasing with up to 20 milliwatts of output power at a heatsink temperature of 77 K, though the output power is highly variable as the reflectance of the output coupler has a strong frequency dependence. At the time of writing this, these are record performances in both frequency tuning and high-temperature continuous wave operation for lasers based on THz QC-gain material. The amount of tuning that be achieved with this approach is limited by the phase response of the metasurface, which squeezes the external cavity modes closer together in the spectral domain. Development of metasurfaces with lower electrical power consumption and higher conversion efficiency for the purpose of improving continuous wave performance. A sparse, patch-based metasurface with reduced power consumption is demonstrated, though the design was not optimal and only showed a 20% reduction in current draw compared to the previously demonstrated metasurfaces. Routes towards improving the performance are discussed. The last subject discussed is the design of a mid-infrared (IR) QC-VECSEL. Due to the large metal losses at mid-IR frequencies compared to THz, the technique used to develop THz QC-VECSELs cannot be directly extended to the mid-IR. We propose a scheme based on a diffraction grating to provide surface coupling of the QC-gain material. Progress on experimental realization is discussed, but lasing has not yet been observed.
Recent advances in Terahertz Quantum Cascade Laser (THz QCL) development are pushing this technology ever closer to practical application, particularly within the spectroscopic field. For this reason, optimizing the operation of THz QCL frequency combs, which can potentially provide unprecedented accuracy and stability to the optical spectra in a broad frequency band, is of particular interest to the research community. The THz QCLs frequency comb was only recently realized using two separate techniques: either a broad-gain active region or a group velocity dispersion controlled waveguide. However, due to residual optical dispersion from both the gain medium and the cold waveguide, comb formation in these reported THz QCLs can only sustain a limited current injection region and the observed comb frequency range is much narrower than the bandwidth of the designed gain medium. To overcome these limitations, this thesis targets a new THz QCL frequency comb device design that simultaneously exploits the broadband gain active region and a group velocity dispersion (GVD)-compensated waveguide over an octave frequency band of 2-4 THz. In designing a broadband gain active region, two heterogeneous structures are proposed and simulated, with one combining three different bound-to-continuum (BTC) active regions operating at a temperature of 25 K, and another one consisting of four different resonant-phonon (RP) active regions operating at the liquid nitrogen temperature (77 K) or higher. The simulation results show that both active region designs can provide a broadband and 'flat-top' gain profile covering the frequency range from 2 to 4 THz. To design a group velocity dispersion-compensated waveguide, strategies are explored for simulating chirped Distributed Bragg Reflectors (DBRs) that can serve as THz QCL metal-metal waveguides, and one-dimensional (1D) and three-dimensional (3D) modeling approaches are established and verified. A novel two-section chirped DBR is proposed, which provides substantially-improved group delay compensation over a broadband octave frequency range from 2 to 4 THz. Two THz QCL structures are grown using in-house molecular beam epitaxy and THz QCL devices equipped with a metal-metal waveguides are fabricated in the University of Waterloo Quantum-Nano-Centre clean-room fabrication lab. The experimental results demonstrate that the new THz QCL active region design can operate up to a maximum lasing temperature of 111 K, and with a broad lasing spectrum covering frequencies from 2.36 to 2.86 THz under pulse mode, at temperature of 13 K. The combined theoretical and experimental work would ultimately lead to the demonstration of improved THz QCL frequency comb operation over the broadband range from 2 to 4 THz.
The invention of optical frequency combs generated by mode-locked lasers revolutionized time and frequency metrology in the late 1990s. This concept has been explored in several laser systems; the quantum cascade laser (QCL) is one such system that operates in the terahertz (THz) frequency range.THz QCL was first invented in 2001 as a reliable semiconductor source for compact, high-power THz radiation. The inherently strong third-order nonlinearity in its QC-gain medium allows for spontaneous frequency comb formation as a result of spatial hole burning induced by Fabry-Perot cavities and four-wave mixing, which synchronizes the dispersed cavity modes. It was noticed that the self-generated combs are naturally frequency-modulated with quasi-continuous power output, whereas amplitude-modulated combs, i.e., mode-locking, are considered challenging in THz QCLs because of the inherent fast gain recovery time. One effective method to trigger active mode-locking is RF injection locking. It involves injecting RF current modulation into the QC-device at a frequency that is close to the cavity round-trip frequency. This locks the spacing between adjacent lasing modes, and pulses with a duration of 4-5 ps have been reported. In recent years, the study of frequency comb/mode-locking in THz QCLs has raised increasing interest because of its potential for a number of applications, including astronomy, biomedicine, fast spectroscopy, non-invasive imaging, and non-destructive evaluation. So far, research has concentrated on ridge-waveguide and ring QCLs. On the other hand, THz quantum-cascade vertical-external-cavity surface-emitting-laser (QC-VECSEL) was introduced in 2015 as a novel external cavity configuration of THz QCLs.The key concept of THz QC-VECSEL is to engineer its gain chip into a millimeter-scale reflectarray metasurface for free-space THz radiation and further incorporation into a resonant laser cavity as an active reflector. This enables watt-level output power with near-Gaussian distributed beam quality; versatile functionality may be incorporated into the amplifying metasurface; and broadband frequency tunability is provided by the VECSEL architecture. Despite the fact that VECSELs are widely used for mode-locking at near-infrared and optical frequencies, THz QC-VECSELs have not yet been exploited in frequency comb and mode-locking applications. In this thesis, we report for the first time the techniques utilized to achieve frequency comb/mode-locking operations in THz QC-VECSELs. Both the metasurface design and VECSEL cavity geometry are optimized for this purpose. The double-patch metasurface design is considered optimal for broadband frequency response and low dispersion, and a well-designed RF package is needed for efficient RF signal injection and extraction. On the other hand, an off-axis parabolic (OAP) mirror is introduced to build a V-shaped intra-cryostat focusing VECSEL cavity. This OAP-focusing cavity design eliminates most of the intra-cavity diffraction losses and, therefore, enables lasing in an ultra-long external cavity using a small-sized metasurface that supports continuous wave (CW) biasing. It is highly suited for frequency comb/mode-locking applications as the cavity round-trip frequency is lowered to a typical value of 3-5 GHz. In contrast to ridge-waveguide or ring QCLs, self-generated frequency combs have not been observed in THz QC-VECSELs --- in fact, they prefer to lase in a single-mode regime primarily due to a lack of spatial hole burning.To promote multimode operation in THz QC-VECSELs, we present a technique based on a specific combination of output coupler thickness and external cavity length. Through Vernier selection and reflectance compensation in a cascaded Fabry-Perot cavity, we are able to perform simultaneous nine modes lasing with a free-spectral range (FSR) of ~21 GHz. The number of lasing modes that can be generated using this method is limited by the maximum available output coupler thickness. A more effective way to promote multimoding, as well as possible frequency comb or even mode-locking operations, is through RF injection locking.The successful demonstration of RF injection locking in THz QC-VECSELs for the first time is the main focus of this thesis. Lasing spectral broadening has been observed under strong RF modulation, with a maximum bandwidth of around 100-300 GHz. An intermodal beat-note is produced as a result of beating between each of the two lasing modes. It is locked to the RF injection signal as the injection frequency is tuned around the cavity round-trip frequency. This suggests that the lasing modes are equally spaced, which is a prerequisite of frequency comb/mode-locking. Several impacting factors, including metasurface design, external cavity length, and optical feedback, are experimentally investigated in the RF-injection locked QC-VECSELs, which may help control and tune the laser states. THz QC-VECSEL is consequently considered to be a superior platform that enables a more thorough investigation of the fundamental physics of mode-locking/frequency comb operation in QCL systems. Our research on mode-locked THz QC-VECSELs opens the way for future development of semiconductor lasers operating in the 2-5 THz region that produce picosecond-scale pulses.
The Encyclopedia of Modern Optics, Second Edition, Five Volume Set provides a wide-ranging overview of the field, comprising authoritative reference articles for undergraduate and postgraduate students and those researching outside their area of expertise. Topics covered include classical and quantum optics, lasers, optical fibers and optical fiber systems, optical materials and light-emitting diodes (LEDs). Articles cover all subfields of optical physics and engineering, such as electro-optical design of modulators and detectors. This update contains contributions from international experts who discuss topics such as nano-photonics and plasmonics, optical interconnects, photonic crystals and 2D materials, such as graphene or holy fibers. Other topics of note include solar energy, high efficiency LED’s and their use in illumination, orbital angular momentum, quantum optics and information, metamaterials and transformation optics, high power fiber and UV fiber lasers, random lasers and bio-imaging. Addresses recent developments in the field and integrates concepts from fundamental physics with applications for manufacturing and engineering/design Provides a broad and interdisciplinary coverage of specialist areas Ensures that the material is appropriate for new researchers and those working in a new sub-field, as well as those in industry Thematically arranged and alphabetically indexed, with cross-references added to facilitate ease-of-use
Room-temperature terahertz (THz) sources analogous to diode lasers in the near-infrared/visible or quantum cascade lasers (QCL) in the mid-infrared (mid-IR), i.e., electrically pumped, compact, widely tunable, and suitable for low-cost production, are highly desired for feasible and inexpensive THz systems. This dissertation focuses on demonstrating broadly tunable, room-temperature THz systems based on intra-cavity difference frequency generation (DFG) in mid-IR QCLs with improved spectral capability for versatile applications. Spectral control using an external cavity provides the widest tuning range and is favored for real-world applications. DFG-THz could be spectrally tuned by either tuning one mid-IR pump or by tuning both mid-IR pumps together. I built a Littrow-type, external cavity THz DFG-QCL system that generated spectral tunable THz radiation by fixing one mid-IR pump frequency with an integrated DFB grating on top of the QCL structure and tuning the other mid-IR pump frequency with an external grating, thus demonstrating record broadband narrow linewidth THz frequency tuning from 1.2 to 5.9 THz. A Cherenkov waveguide is used in this system to extract THz radiation through the semi-insulating InP substrate; however, InP has dispersion in 1–6 THz, resulting in steering far field profiles for different THz frequencies. Replacing the InP substrate with high-resistance silicon through an adhesive bonding process solved the beam steering problem of this THz DFG-QCL system. I also built a double-Littrow, external cavity DFG-THz system that tunes both mid-IR pump frequencies using two external diffraction gratings. Such a system allows performing a comprehensive spectroscopic study of the optical nonlinearity and its dependence on the mid-infrared pump frequencies. Our work shows that the terahertz generation efficiency can vary by a factor of two or more, depending on the spectral position of the mid-infrared pumps, even for a fixed THz difference frequency. Using this system, we investigated different active region designs: bound-to-continuum, continuum-to-continuum, three-phonon-resonance, and dual-upper-state active region design. Our studies show THz DFG-QCL based a bound-to-continuum active region with gain centered around 15 μm has an order of magnitude enhancement of mid-IR to THz conversion efficiency, which provides a trend for future improvement of the power performance of THz DFG-QCLs